Third-order nonlinear Hall effect induced by the Berry-connection polarizability tensor

نویسندگان

چکیده

Nonlinear responses in transport measurements are linked to material properties not accessible at linear order1 because they follow distinct symmetry requirements2–5. While the Hall effect indicates time-reversal breaking, second-order nonlinear typically requires broken inversion symmetry1. Recent experiments on ultrathin WTe2 demonstrated this connection between crystal structure and response6,7. The observed can probe Berry curvature dipole, a band geometric property, non-magnetic materials, just like anomalous probes magnetic materials8,9. Theory predicts that another intrinsic Berry-connection polarizability tensor10, gives rise higher-order signals, but it has been probed experimentally. Here, we report third-order thick Td-MoTe2 samples. signal is found be dominant response over both linear- ones. Angle-resolved reveal feature results from constraints. Temperature-dependent measurement shows agrees with contribution evaluated by first-principles calculations. provides valuable for intriguing lower orders may employed high-order-response electronic devices. unveil specific measurements. In samples, dominates lower-order contributions tensor.

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ژورنال

عنوان ژورنال: Nature Nanotechnology

سال: 2021

ISSN: ['1748-3395', '1748-3387']

DOI: https://doi.org/10.1038/s41565-021-00917-0